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Light2Hydrogen Publications

The following publications have evolved from the L2H research field at the TUB:

2014

  • Applying thermo-destabilization of microemulsions as a new method for co-catalyst loading on mesoporous polymeric carbon nitride – towards large scale applications
    Marc Schröder, Kamalakannan Kailasam, Stefan Rudi, Kyonmin Fündling, Julian Rieß, Michael Lublow, Arne Thomas, Reinhard Schomäcker, Michael Schwarze
    RSC Adv. 2014, 4, 50017-50026   link

  • Impact of the reaction conditions on the photocatalytic reduction of water on mesoporous polymeric carbon nitride under sunlight irradiation
    Marc Schröder, Kamalakannan Kailasam, Stefan Rudi, Marcel Richter, Arne Thomas, Reinhard Schomäcker, Michael Schwarze
    Int. J. Hydrogen Energy 2014, 39, 10108-10120   link

  • Visible light driven non-sacrificial water oxidation and dye degradation with silver phosphates: multi-faceted morphology matters
    Arindam Indra, Prashanth W. Menezes, Michael Schwarze, Matthias Driess
    New J. Chem. 2014, 38, 1942-1945   link

  • Nanostructured Manganese Oxides as Highly Active Water Oxidation Catalysts: A Boost from Manganese Precursor Chemistry
    Prashanth W. Menezes, Arindam Indra, Patrick Littlewood, Michael Schwarze, Caren Göbel, Reinhard Schomäcker, Matthias Driess
    ChemSusChem 2014, 7, 2202-2211   link

  • Polymeric Carbon Nitride/Mesoporous Silica Composites as Catalyst Support for Au and Pt Nanoparticles
    Ping Xiao, Yanxi Zhao, Tao Wang, Yingying Zhan, Huihu Wang, Jinlin Li, Arne Thomas, Junjiang Zhu

    Chem. Eur. J. 2014, 20, 2872-2878   link

  • A Molecular Approach to Self-Supported Cobalt-Substituted ZnO Materials as Remarkably Stable Electrocatalysts for Water Oxidation
    Johannes Pfrommer, Michael Lublow, Anahita Azarpira, Caren Göbel, Marcel Lücke, Alexander Steigert, Martin Pogrzeba, Prashanth W. Menezes, Anna Fischer, Thomas Schedel-Niedrig, Matthias Driess
    Angew. Chem. Int. Ed. 2014, 53, 5183-5187   link

  • Structure–Activity Relationships in Bulk Polymeric and Sol–Gel-Derived Carbon Nitrides during Photocatalytic Hydrogen Production
    Dirk Hollmann, Michael Karnahl, Stefanie Tschierlei, Kamalakannan Kailasam, Matthias Schneider, Jörg Radnik, Kathleen Grabow, Ursula Bentrup, Henrik Junge, Matthias Beller, Stefan Lochbrunner, Arne Thomas, Angelika Brückner
    Chem. Mater.
    2014, 26, 1727-1733   link
  • THF: An Efficient Electron Donor in Continuous Flow Radical Cyclization Photocatalyzed by Graphitic Carbon Nitride
    Magdalena Woźnica, Nicolas Chaoui, Soraya Taabache, Siegfried Blechert
    Chem. Eur. J. 2014, 20, 14624–14628   link

  • Carbon Nitride-Catalyzed Photoredox Sakurai Reactions and Allylborations
    Lennart Möhlmann, Siegfried Blechert
    Adv. Synth. Catal. 2014, 356, 2825-2829   link

2013

  • Active Mixed-Valent MnOx Water Oxidation Catalysts through Partial Oxidation (Corrosion) of Nanostructured MnO Particles
    Arindam Indra, Prashanth W. Menezes, Ivelina Zaharieva, Elham Baktash, Johannes Pfrommer, Michael Schwarze, Holger Dau, Matthias Driess
    Angew. Chem. Int. Ed. 2013, 52, 13206-13210   link

  • Room Temperature Synthesis of Heptazine-Based Microporous Polymer Networks as Photocatalysts for Hydrogen Evolution
    Kamalakannan Kailasam, Johannes Schmidt, Hakan Bildirir, Guigang Zhang, Siegfried Blechert, Xinchen Wang, Arne Thomas
    Macromol. Rapid Commun. 2013, 34, 1008-1013   link

  • Three-Dimensional Macroscopic Assemblies of Low-Dimensional Carbon Nitrides for Enhanced Hydrogen Evolution
    Young-Si Jun, Jihee Park, Sun Uk Lee, Arne Thomas, Won Hi Hong, Galen D. Stucky
    Angew. Chem. Int. Ed. 2013, 52, 11083-11087   link

  • From Melamine-Cyanuric Acid Supramolecular Aggregates to Carbon Nitride Hollow Spheres
    Young-Si Jun, Eun Zoo Lee, Xinchen Wang, Won Hi Hong, Galen D. Stucky, Arne Thomas
    Adv. Funct. Mater. 2013, 23, 3661-3667   link

  • A One-Pot Approach to Mesoporous Metal Oxide Ultrathin Film Electrodes Bearing One Metal Nanoparticle per Pore with Enhanced Electrocatalytic Properties
    Amandine Guiet, Tobias Reier, Nina Heidary, Diana Felkel, Benjamin Johnson, Ulla Vainio, Helmut Schlaad, Yilmaz Aksu, Matthias Driess, Peter Strasser, Arne Thomas, Jörg Polte, Anna Fischer
    Chem. Mater.
    2013, 25, 4645-4652   link

  • Exfoliation of Crystalline 2D Carbon Nitride: Thin Sheets, Scrolls and Bundles via Mechanical and Chemical Routes
    Michael J. Bojdys, Nikolai Severin, Jürgen P. Rabe, Andrew I. Cooper, Arne Thomas, Markus Antonietti
    Macromol. Rapid Commun. 2013, 34, 850-854   link

  • Electro- and Photochemical Water Oxidation on Ligand-free Co3O4 Nanoparticles with Tunable Sizes   
    Marek Grzelczak, Jinshui Zhang, Johannes Pfrommer, Jürgen Hartmann, Matthias Driess, Markus Antonietti, Xinchen Wang
    ACS Catal. 2013, 3, 383-388   link

  • NHC-catalysed highly selective aerobic oxidation of nonactivated aldehydes
    Lennart Möhlmann, Stefan Ludwig, Siegfried Blechert
    Beilstein J. Org. Chem. 2013, 9, 602–607   link

  • Facilitating room-temperature Suzuki coupling reaction with light: Mott-Schottky photocatalyst for C-C-coupling
    Xin-Hao Li, Moritz Baar, Siegfried Blechert, Markus Antonietti
    Scientific Reports 2013, 3, 1743   link

  • Entwicklung eines Reaktors zur standardisierten Quantifizierung der photokatalytischen Wasserstofferzeugung (Development of a Reactor for Standardized Quantification of the Photocatalytic Hydrogen Production)
    Michael Schwarze, Marc Schröder, Diana Stellmach, Kamalakannan Kailasam, Arne Thomas, Reinhard Schomäcker
    Chem. Ing. Tech. 2013, 85, 500-507   link

  • Quantification of photocatalytic hydrogen evolution
    Michael Schwarze, Diana Stellmach, Marc Schröder, Kamalakannan Kailasam, Rulle Reske, Arne Thomas, Reinhard Schomäcker
    Phys. Chem. Chem. Phys. 2013, 15, 3466–3472   link

2012

  • Metal-Free Photocatalytic Graphitic Carbon Nitride on p-Type Chalcopyrite as a Composite Photocathode for Light-Induced Hydrogen Evolution
    Florent Yang, Michael Lublow, Steven Orthmann, Christoph Merschjann, Tobias Tyborski, Marin Rusu, Sven Kubala, Arne Thomas, Rosa Arrigo, Michael Hävecker, Thomas Schedel-Niedrig
    ChemSusChem 2012, 5, 1227–1232   link

  • Carbon Nitride-Catalyzed Photoredox CC Bond Formation with N-Aryltetrahydroisoquinolines
    Lennart Möhlmann, Moritz Baar, Julian Rieß, Markus Antonietti, Xinchen Wang, Siegfried Blechert
    Adv. Synth. Catal
    . 2012, 354, 1909–1913   link

  • Co-Monomer Control of Carbon Nitride Semiconductors to Optimize Hydrogen Evolution with Visible Light
    Jinshui Zhang, Guigang Zhang, Xiufang Chen, Lin Sen, Lennart Möhlmann, Grzegorz Dolega, Grzegorz Lipner, Markus Antonietti, Siegfried Blechert, Xinchen Wang
    Angew. Chem. Int. Ed. 2012, 51, 3183–3187   link

  • Polymeric Graphitic Carbon Nitride for Heterogeneous Photocatalysis
    Xinchen Wang, Siegfried Blechert, Markus Antonietti
    ACS Catal.
    2012, 2, 1596
    1606   link

2011

  • Mesoporous carbon nitride–silica composites by a combined solgel/thermal condensation approach and their application as photocatalysts
    Kamalakannan Kailasam, Jan Dirk Epping, Arne Thomas, Sebastian Losse, Henrik Junge
    Energy Environ.
    Sci.
    20114, 4668–4674   link

  • Condensed Graphitic Carbon Nitride Nanorods by Nanoconfinement: Promotion of Crystallinity on Photocatalytic Conversion
    Xin-Hao Li, Jinshui Zhang, Xiufang Chen, Anna Fischer, Arne Thomas, Markus Antonietti, Xinchen Wang
    Chem. Mater.
    2011, 23, 4344–4348   link

  • Surface photovoltage spectroscopy of carbon nitride powder
    Th. Dittrich, S. Fiechter, A. Thomas
    Appl. Phys.
    Lett.
    2011, 99, 084105   link

  • A Molecular Precursor Approach to Tunable Porous Tin-Rich Indium Tin Oxide with Durable High Electrical Conductivity for Bioelectronic Devices
    Yilmaz Aksu, Stefano Frasca, Ulla Wollenberger, Matthias Driess, Arne Thomas
    Chem. Mater. 2011, 23, 1798–1804   link

  • Aerobic Oxidative Coupling of Amines by Carbon Nitride Photocatalysis with Visible Light
    Fangzheng Su, Smitha C. Mathew, Lennart Möhlmann, Markus Antonietti, Xinchen Wang, Siegfried Blechert
    Angew.
    Chem. Int. Ed. 201150, 657–660   link

2010

  • Cubic Mesoporous Graphitic Carbon(IV) Nitride: An All-in-One Chemosensor for Selective Optical Sensing of Metal Ions
    Eun Zoo Lee, Young-Si Jun, Won Hi Hong, Arne Thomas, Moonsoo M. Jin
    Angew. Chem. Int. Ed. 2010, 49, 9706-9710   link

  • Making MetalCarbon Nitride Heterojunctions for Improved Photocatalytic Hydrogen Evolution with Visible Light
    Yan Di, Xinchen Wang, Arne Thomas, Markus Antonietti
    ChemCatChem 2010, 2, 834–838   link
  • Ionothermal Route to Layered Two-Dimensional Polymer-Frameworks Based on Heptazine Linkers
    Michael J. Bojdys, Stephanie A. Wohlgemuth, Arne Thomas, Markus Antonietti
    Macromolecule,
    2010, 43, 6639–6645   link

  • mpg-C3N4-Catalyzed Selective Oxidation of Alcohols Using O2 and Visible Light
    Fangzheng Su, Smitha C. Mathew, Grzegorz Lipner, Xianzhi Fu, Markus Antonietti, Siegfried Blechert, Xinchen Wang
    J. Am. Chem. Soc. 2010132, 16299-16301   link

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L2H Office Berlin
Prof. Dr. Michael Schwarze
Technische Universitaet Berlin
Institute of Process Engineering
sec. TK 01
Strasse des 17. Juni 135
10623 Berlin
tel. +49 30 314-26964
or -24097